Issue |
E3S Web Conf.
Volume 213, 2020
2nd International Conference on Applied Chemistry and Industrial Catalysis (ACIC 2020)
|
|
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Article Number | 01002 | |
Number of page(s) | 5 | |
Section | Industrial Catalysis and Chemical Substance R&D and Application | |
DOI | https://doi.org/10.1051/e3sconf/202021301002 | |
Published online | 01 December 2020 |
Investigation of Chemical-looping Gasification Characteristics of Chinese Western Coals with Hematite-CuO Oxygen Carrier
1
State Key Laboratory of High-efficiency Coal Utilization and Green Chemical Engineering, School of Chemistry and Chemical Engineering, Ningxia University, Yinchuan, 750021, China
2
Key Laboratory of Coal Processing and Efficient Utilization, Ministry of Education, China University of Mining & Technology, Xuzhou 221116, Jiangsu, China
3
NingXia Vocational Technical College Of Industry And Commerce, Yinchun, 750021, China
* Corresponding author: qj_guo@yahoo.com
In order to realize highly efficient conversion of Chinese western bituminous coals into syngas, a series of chemical-looping gasification experiments was conducted with hematite-CuO oxygen carrier in a laboratory-scale fluidized-bed reactor. The results indicated that the gasification rate of Chinese western bituminous increased by 2-3 times after addition of a hematite-CuO oxygen carrier. Meanwhile, the syngas yields of Chinese western bituminous ranged from 1.84–2.04 m3/kg, three times higher than that of lignite. This shows that the combination of chemical-looping technology and gasification of coal can achieve efficient conversion of Chinese/western bituminous coals. The temperature and the supply oxygen coefficient (O/C) all demonstrated a clear effect on the gasification rates and the gas yields. 10 cycles of redox experiments indicated that the hematite-CuO oxygen carriers have good recycled reaction characteristics. Those results provide theoretical guidance for the efficient conversion of Chinese western bituminous coals into syngas via chemical-looping gasification.
© The Authors, published by EDP Sciences, 2020
This is an Open Access article distributed under the terms of the Creative Commons Attribution License 4.0, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
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